Berry curvature of low-energy excitons in rhombohedral graphene
H. Davenport, F. Schindler, J. Knolle
Physical Review B 113 (11), 115102 (2026).
We investigate low-energy excitons in rhombohedral pentalayer graphene encapsulated by hexagonal boron nitride (hBN/R5G/hBN), focusing on the regime at the experimental twist angle theta = 0.77 degrees and with an applied electric field. We introduce a new low-energy two-band model of rhombohedral graphene that captures the band structure more accurately than previous models while keeping the number of parameters low. Using this model, we show that the centres of the exciton Wannier functions are displaced from the moir & eacute,. unit cell origin by a quantized amount-they are instead localized at C3-symmetric points on the boundary. We also find that the exciton shift is electrically tunable: by varying the electric field strength, the exciton Wannier center can be exchanged between inequivalent corners of the moir & eacute,. unit cell. Our results suggest the possibility of detecting excitonic corner or edge modes, as well as novel excitonic crystal defect responses in hBN/R5G/hBN. Lastly, we find that the excitons in hBN/R5G/hBN inherit excitonic Berry curvature from the underlying electronic bands, enriching their semiclassical transport properties. Our results position rhombohedral graphene as a compelling tunable platform for probing exciton topology in moir & eacute,. materials.
Prethermalization by random multipolar driving on a 78-qubit processor
Z.-H. Liu, Y. Liu, G.-H. Liang, C.-L. Deng, K. Chen, Y.-H. Shi, T.-M. Li, L. Zhang, B.-J. Chen, C.-P. Fang, D. e. Feng, X.-Y. Gu, Y. He, K. Huang, H. Li, H.-T. Liu, L. Li, Z.-Y. Mei, Z.-Y. Peng, J.-C. Song, M.-C. Wang, S.-L. Wang, Z. Wang, Y. Xiao, M. Xu, Y.-S. Xu, Y. Yan, Y.-H. Yu, W.-P. Yuan, J.-C. Zhang, J.-J. Zhao, K. Zhao, S.-Y. Zhou, Z.-A. Wang, X. Song, Y. Tian, F. Mintert, J. Knolle, R. Moessner, Y.-R. Zhang, P. Zhang, Z. Xiang, D. Zheng, K. Xu, H. Zhao, H. Fan
Nature 650 (8100), (2026).
Time-dependent drives hold promise for realizing non-equilibrium many-body phenomena that are absent in undriven systems1, 2-3. Yet, drive-induced heating normally destabilizes the systems4,5, which can be parametrically suppressed in the high-frequency regime by using periodic (Floquet) drives6,7. It remains largely unknown to what extent highly controllable quantum simulators can suppress heating in non-periodically driven systems. Here, using the 78-qubit superconducting quantum processor, Chuang-tzu 2.0, we report the experimental observation of long-lived prethermal phases in many-body systems with tunable heating rates, driven by structured random protocols, characterized by n-multipolar temporal correlations. By measuring both the particle imbalance and subsystem entanglement entropy, we monitor the entire heating process over 1,000 driving cycles and observe the existence of the prethermal plateau. The prethermal lifetime is 'doubly tunable': one way by driving frequency, the other way by multipolar order,. it grows algebraically with the frequency with the universal scaling exponent 2n + 1. Using quantum-state tomography on different subsystems, we demonstrate a non-uniform spatial entanglement distribution and observe a crossover from area-law to volume-law entanglement scaling. With 78 qubits and 137 couplers in a two-dimensional configuration, the entire far-from-equilibrium heating dynamics are beyond the reach of simulation using tensor-network numerical techniques. Our work highlights superconducting quantum processors as a powerful platform for exploring universal scaling laws and non-equilibrium phases of matter in driven systems in regimes where classical simulation faces formidable challenges.
Altermagnetism without crystal symmetry
P. D'Ornellas, V. Leeb, A. G. Grushin, J. Knolle
Physical Review B 113 (2), 24426 (2026).
Altermagnetism is a collinear magnetic order in which opposite spin species are exchanged under a real-space rotation. Hence, the search for physical realizations has focused on crystalline solids with specific rotational symmetry. Here, we show that altermagnetism can also emerge in noncrystalline systems, such as amorphous solids, despite the lack of global rotational symmetries. We construct a minimal Hamiltonian with two directional orbitals per site on an amorphous lattice with interactions that are invariant under spin rotation. Altermagnetism then arises due to spontaneous symmetry breaking in the spin and orbital degrees of freedom around each atom, displaying a common point group symmetry. This form of altermagnetism exhibits anisotropic spin transport and spin spectral functions, both experimentally measurable. Our mechanism generalizes to any lattice and any altermagnetic order, opening the search for altermagnetic phenomena to noncrystalline systems.
Exciton Berryology
H. Davenport, J. Knolle, F. Schindler
Physical Review B 113 (4), 45125 (2026).
In translationally invariant semiconductors that host exciton bound states, one can define an infinite number of possible exciton Berry connections. These correspond to the different ways in which a many-body exciton state, at fixed total momentum, can be decomposed into free electron and hole Bloch states that are entangled by an exciton envelope wave function. Inspired by the modern theory of polarization, we define an exciton projected position operator whose eigenvalues single out two unique choices of exciton Berry phase and associated Berry connection-one for electrons, and one for holes. We clarify the physical meaning of these exciton Berry phases and provide a discrete Wilson loop formulation that allows for their numerical calculation without a smooth gauge. As a corollary, we obtain a gauge-invariant expression for the exciton polarization at a given total momentum, i.e., the mean separation of the electron and hole within the exciton wave function. In the presence of crystalline inversion symmetry, the electron and hole exciton Berry phases are quantized to the same value and we derive how this value can be expressed in terms of inversion eigenvalues of the many-body exciton state. We then consider C2T symmetry, for which no symmetry eigenvalues are available as it is antiunitary, and confirm that the exciton Berry phase remains quantized and still diagnoses topologically distinct exciton bands. The notion of shift excitons, whose exciton Wannier states are displaced from those of the noninteracting bands by a quantized amount, can therefore be generalized beyond symmetry indicators.
Quantum critical dynamical response of the twisted Kitaev spin chain
U. E. Khodaeva, D. L. Kovrizhin, J. Knolle
Physical Review B 113 (4), 45120 (2026).
The dynamical structure factor of the transverse field Ising model (TFIM) shows universal power-law divergence at its quantum critical point, signatures of which have been arguably observed in inelastic neutron scattering studies of quantum spin chain materials, for example CoNb2O6. However, it has recently been suggested that its microscopic description is better captured in terms of a twisted Kitaev spin chain (TKSC) with bond-anisotropic couplings. Here, we present exact results for the dynamical structure factor of the TKSC across its quantum critical point, analyzing both the universal low-frequency response and the non-universal high-energy features. In addition, we explore extensions of the model including broken glide symmetry as well as the case of random, and incommensurate magnetic fields. Notably, in the latter case, the fermionic excitations exhibit a localization-delocalization transition, which is manifest in the dynamical response as a distinct signature at finite frequency. We discuss the relevance of these features for the observation of quantum critical response in experiments.
Projectively Implemented Altermagnetism in an Exactly Solvable Quantum Spin Liquid
A. Neehus, A. Rosch, J. Knolle, U. F. P. Seifert
Physical Review Letters 135 (25), 256504 (2025).
"Altermagnets are a new class of symmetry-compensated magnets with large spin splittings. Here, we show that the notion of altermagnetism extends beyond the realm of Landau-type order: we study exactly solvable Z2 quantum spin(-orbital) liquids (QSLs), which simultaneously support magnetic long-range order as well as fractionalization and Z2 topological order. Our symmetry analysis reveals that in this model three distinct types of ""fractionalized altermagnets (AM*)"" emerge, which can be distinguished by their residual symmetries. Importantly, the fractionalized excitations of these states carry an emergent Z2 gauge charge, which implies that they transform projectively under symmetry operations. Consequently, we show that ""altermagnetic spin splittings"" are now encoded in a momentum-dependent particle-hole asymmetry of the fermionic parton bands. We discuss consequences for experimental observables such as dynamical spin structure factors and (nonlinear) thermal and spin transport."
Van Hove singularities and competing instabilities in an altermagnetic metal
P. Rao, J. Knolle, L. Classen
Physical Review B 112 (23), 235140 (2025).
Van Hove (VH) singularities in the single-particle band spectrum are important for interaction-driven quantum phases. Whereas VH points are usually spin-degenerate, in newly proposed altermagnets VH singularities can become spin-dependent, due to momentum-dependent spin polarization of the Fermi surfaces arising from combined rotation and time-reversal symmetry. We consider two altermagnetic models (dx2-y2- and dxy-wave) on a square lattice with spin-polarized VH points, and study their stable fixed-point solutions indicating interaction-induced instabilities using parquet renormalization group. For both models, we find new stable fixed-point solutions of the renormalization group equations which are not connected to the solution in the spin-degenerate limit. This implies that on the square lattice, the system with VH singularities is unstable with respect to altermagnetic perturbations. The leading instability for the dx2-y2 model is real transverse spin density wave. For the dxy-wave model, it is found to be real transverse spin density wave at large altermagnetic splitting. At small altermagnetic splitting both imaginary charge density wave and real longitudinal spin density waves are dominant.
Stability of algebraic spin liquids coupled to quantum phonons
F. Ferrari, J. Willsher, U. F. P. Seifert, R. Valenti, J. Knolle
Physical Review Research 7 (4), L042053 (2025).
Algebraic spin liquids are quantum disordered phases of insulating magnets that exhibit fractionalized gapless excitations and power-law correlations. Quantum spin liquids in this category include the experimentally established one-dimensional (1D) Luttinger liquid, as well as the U(1) Dirac spin liquid (DSL) that has been a focus of recent candidate materials searches. Most notably, several exchange-frustrated Heisenberg materials on the triangular lattice have shown evidence of the U(1) DSL. In this work, we measure the algebraic correlations of spin-singlet excitations in the J1-J2 antiferromagnetic Heisenberg model on the triangular lattice, prompting a detailed investigation of this model's stability under spin-lattice coupling with dynamical quantum phonons using variational Monte Carlo. As seen before in 1D spin chains, we observe a low-temperature transition from a U(1) DSL to valence bond order and predict the parameter regime where the model realizes a stable DSL ground state. To achieve this, we employ a series of finite-size scaling Ans & auml,.tze inspired by the low-energy DSL's conformal description in terms of quantum electrodynamics and show that emergent monopole operators drive the instability. We compare the physics of this transition to the 1D Luttinger liquid throughout our analysis. We derive the regime of stability against spin-Peierls ordering and argue that the DSL ground state might still be achievable in candidate materials, despite its tendency to valence bond solid ordering.
Fractionalized prethermalization in the one-dimensional Hubbard model
A. Romen, J. Knolle, M. Knap
Physical Review B 112 (19), 195124 (2025).
Prethermalization phenomena in driven systems are generally understood via a local Floquet Hamiltonian obtained from a high-frequency expansion. Remarkably, recently it has been shown that a driven Kitaev spin liquid with fractionalized excitations can realize a quasistationary state that is not captured by this paradigm. Instead distinct types of fractionalized excitations are characterized by vastly different temperatures-a phenomenon dubbed fractionalized prethermalization. In our work, we analyze fractionalized prethermalization in a driven one-dimensional Hubbard model at strong coupling which hosts spin-charge fractionalization. At intermediate frequencies quasisteady states emerge which are characterized by a low spin and high charge temperature with lifetimes set by two competing processes: the lifetime of the quasiparticles determined by Fermi's Golden rule and the exponentially long lifetime of a Floquet prethermal plateau. We classify drives into three categories, each giving rise to distinct (fractional) prethermalization dynamics. Resorting to a time-dependent variant of the Schrieffer-Wolff transformation, we systematically analyze how these drive categories are linked to the underlying driven Hubbard model, thereby providing a general understanding of the emergent thermalization dynamics. We discuss routes toward an experimental realization of this phenomenon in quantum simulation platforms.
Experimental observation of a time rondeau crystal
L. J. Il Moon, P. M. Schindler, Y. Sun, E. Druga, J. Knolle, R. Moessner, H. Zhao, M. Bukov, A. Ajoy
Nature Physics 21 (11), (2025).
Conventional phases of matter can be characterized by the symmetries they break, one example being water ice whose crystalline structure breaks the continuous translation symmetry of space. Recently, breaking of time-translation symmetry was observed in non-equilibrium systems, producing so-called time crystals. Here we investigate different kinds of partial temporal ordering, stabilized by non-periodic yet structured drives, which we call the rondeau order. Using carbon-13 nuclear spins in diamond as a quantum simulator, we use microwave driving fields to create tunable short-time disorder in a system exhibiting long-time stroboscopic order. Our spin control architecture allows us to implement a family of driving fields including periodic, aperiodic and structured random drives. We use a high-throughput read-out scheme to continuously observe the spin polarization and its rondeau order, with controllable lifetimes exceeding 4 s. Using degrees of freedom associated with the short-time temporal disorder of rondeau order, we demonstrate the capacity to encode information in the response of observables. Our work broadens the landscape of observed non-equilibrium temporal order, and raises the prospect for the potential applications of driven quantum matter.
Order-by-disorder in magnets with frustrated spin interactions-classical and large-S limits via the spin functional integral
P. Rao, J. Knolle
Journal of Physics-Condensed Matter 37 (40), 405802 (2025).
We investigate spin systems with extensive degeneracies in the classical ground states due to anisotropic frustrated spin interactions, where the degeneracy is not protected by symmetry. Using spin functional integration, we study the lifting of the degeneracies by fluctuations called order-by-disorder (ObD), and the associated gap in the spin-wave spectrum. It is shown that ObD corresponds to gradient-dependent anisotropic interactions of the pseudo-Goldstone modes, which vanish for a classical uniform spin configuration. Fluctuations generate a gradient-independent effective potential which determines the ground state and the pseudo-Goldstone gap. Furthermore, we recover previous predictions for the pseudo-Goldstone gap in type-I and II ObD with two-spin interactions in the large spin-S limit or the classical small temperature limit, by computing the gap explicitly for the type-II cubic compass model and the type-I square compass model. We show that these two limits correspond to the one-loop approximation for the effective potential. We also discuss other types of order by disorder due to m-spin interactions where m > 2.
Exploring d-wave magnetism in cuprates from oxygen moments
Y. Li, V. Leeb, K. Wohlfeld, R. Valenti, J. Knolle
Physical Review B 112 (12), 125139 (2025).
The antiferromagnetic parent phase of high-Tc cuprates has been established as a N & eacute,.el state of copper moments, but early work pointed out the important role of ligand oxygen orbitals. Using the three-orbital Emery model, we explore how, and under which conditions, doping-induced antiferromagnetic ordering of weak magnetic moments on the oxygen sites can lead to unconventional d-wave magnetism with spin-split electronic bands. The mechanism for forming such altermagnetic (AM) states in cuprates does not rely on a lowering of the crystal symmetry but rather on interaction-induced formation of magnetic moments on directional oxygen orbitals within the crystallographic unit cell. Therefore, we obtain two different types of AM, namely, a (0, 0)-AM and a (pi, pi)-AM. We explore different regimes and challenges for realizing oxygen AM supported by Hartree-Fock calculations and complementary exact diagonalization of small clusters. While the region of interacting parameters needed to realize these states may be difficult to achieve in known high-Tc cuprates, we propose a scenario to realize AM induced by oxygen magnetic moments in a cuprate-based candidate compound using density functional theory and discuss experimental implications.
Genuine Topological Anderson Insulator from Impurity Induced Chirality Reversal
A. Neehus, F. Pollmann, J. Knolle
Physical Review Letters 135 (12), 126604 (2025).
We investigate a model of Dirac fermions with mass impurities that open a global topological gap even in the dilute limit. Surprisingly, we find that the chirality of this mass term, i.e., the sign of the Chern number, can be reversed by tuning the magnitude of the single-impurity scattering. Consequently, the disorder induces a phase disconnected from the simple clean limit of the topological insulator, which is achieved via an impurity resonance inducing additional bands with Chern number 2. Thus, we call this impurity induced phase a genuine topological Anderson insulator. In seeming contradiction to the expectation that mass disorder is an irrelevant perturbation to the Dirac semimetal, the tricritical point separating these two Chern insulating phases and a thermal metal phase is located at zero impurity density and connected to the appearance of a zero energy bound state in the continuum that corresponds to a perfectly resonant mass impurity. Our conclusions based on the T-matrix expansion are substantiated by large scale Chebyshevpolynomial Green's function numerics. We discuss possible experimental platforms.
Scattering theory of chiral edge modes in topological magnon insulators
S. Birnkammer, M. Knap, J. Knolle, A. Mook, A. Bastianello
Physical Review B 112 (9), 94417 (2025).
Topological magnon insulators exhibit robust edge modes with chiral properties similar to quantum Hall edge states. However, due to their strong localization at the edges, interactions between these chiral edge magnons can be significant, as we show in a model of coupled magnon-conserving spin chains in an electric field gradient. The chiral edge modes remain edge-localized and do not scatter into the bulk, and we characterize their scattering phase: for strongly localized edge modes, we observe significant deviation from the bare scattering phase. This renormalization of edge scattering can be attributed to bound bulk modes resonating with the chiral edge magnons in the spirit of Feshbach resonances in atomic physics. We argue that the scattering dynamics can be probed experimentally with a real-time measurement protocol using inelastic scanning tunneling spectroscopy. Our results show that interaction among magnons can be encoded in an effective edge model of reduced dimensionality, where the interactions with the bulk renormalize the effective couplings. Our work introduces a systematic way to determine the many-body effective theory for edge states in topological magnon insulators.
Dynamical response theory of interacting Majorana fermions and its application to generic Kitaev quantum spin liquids in a field
P. Rao, R. Moessner, J. Knolle
Physical Review B 112 (2), 24440 (2025).
"Motivated by the appearance of Majorana fermions in a broad range of correlated and topological electronic systems, we develop a general method to compute the dynamical response of interacting Majorana fermions in the random-phase approximation (RPA). This can be applied self-consistently on top of Majorana mean-field theory backgrounds, thereby in particular providing a powerful tool to analyze generic behavior in the vicinity of (various heavily studied) exactly soluble models. Prime examples are quantum spin liquids (QSL) with emergent Majorana excitations, with the celebrated exact solution of Kitaev. We employ the RPA to study in considerable detail phase structure and dynamics of the extended Kitaev honeycomb KJP model, with and without an applied field. First, we benchmark our method with Kitaev's exactly soluble model, finding a remarkable agreement. The interactions between Majorana fermions even turn out to mimic the effect of local Z2 flux excitations, which we explain analytically. Second, we show how small non-Kitaev couplings J and P induce Majorana bound states, resulting in sharp features in the dynamical structure factor in the presence of fractionalization: such ""spinon excitons"" naturally appear, and can coexist and interact with the broad Majorana continuum. Third, for increasing couplings or field, our theory predicts instabilities of the Kitaev QSL (KQSL) triggered by the condensation of the sharp modes. From the high-symmetry momenta of the condensation we can deduce which magnetically ordered phases surround the KQSL, in good agreement with previous finite-size numerics. We discuss implications for experiments and the broad range of applicability of our method to other QSL and Majorana systems."
Genuine quantum scars in many-body spin systems
A. Pizzi, L.-H. Kwan, B. Evrard, C. B. Dag, J. Knolle
Nature Communications 16 (1), 6722 (2025).
Chaos makes isolated systems of many interacting particles quickly thermalize and forget about their past. Here, we show that quantum mechanics hinders chaos in many-body systems: although the quantum eigenstates are thermal and strongly entangled, exponentially many of them are scarred, that is, have an enlarged weight along underlying classical unstable periodic orbits. Scarring makes the system more likely to be found on an orbit it was initialized on, retaining a memory of its past and thus weakly breaking ergodicity, even at long times and despite the system being fully thermal and the eigenstate thermalization hypothesis fulfilled. We demonstrate the ubiquity of quantum scarring in many-body systems by considering a large family of spin models, including some of the most popular ones from condensed matter physics. Our findings, at hand for modern quantum simulators, prove structure in spite of chaos in many-body quantum systems. Chaos causes interacting particles to rapidly thermalize and lose memory of their past. Here, the authors show that, despite thermalization, genuine quantum scarring can imprint structure and long-lived memory effects in the many-body wavefunction.
Pair density waves and supercurrent diode effect in altermagnets
G. Sim, J. Knolle
Physical Review B 112 (2), L020502 (2025).
Metallic altermagnets are unusual collinear magnets that feature zero net magnetization with momentum-dependent spin splitting. Here, we show that this spin splitting can induce pair density wave states even in the absence of external magnetic fields. Focusing on BCS-type attractive interactions, we find the stabilization of symmetrically distinct pair density wave states depending on the chemical potential. These states include Fulde-Ferrell and Fulde-Ferrell* states, both of which break inversion symmetry. We investigate the supercurrent properties and discover nonreciprocal supercurrents for both the Fulde-Ferrell and Fulde-Ferrell* states with distinct spatial dependencies. We propose that the supercurrent diode effect can serve as an experimental tool for distinguishing between different pair density waves in metallic altermagnets and discuss the relation to material candidates.
Ferrimagnetic Kitaev spin liquids in mixed spin-1/2 and spin-3/2 honeycomb magnets
W. Natori, Y. Yang, H.-K. Jin, J. Knolle, N. B. Perkins
Physical Review B 111 (21), 214411 (2025).
We explore the phase diagram of a mixed-spin Kitaev model, where spin-1/2 and spin-3/2 ions form a staggered pattern on a honeycomb lattice. Enabled by an exact mapping of local conserved flux operators onto Z2 gauge fields, we perform a parton mean-field theory for the model with a single-ion anisotropy. The phase diagram contains four types of quantum spin liquids distinguished by quadrupolar parameters. These analytical results are quantitatively confirmed by state-of-the-art DMRG simulations. We also explore the potential experimental realization of the mixed-spin Kitaev model in materials such as Zr0.5Ru0.5Cl3. By developing a superexchange theory specifically for this mixed-spin system, we identify the conditions under which dominant Kitaev-like interactions emerge. Our findings highlight the importance of spin-orbital couplings and quadrupolar order parameters in stabilizing exotic phases, providing a foundation for exploring mixed-spin Kitaev magnets.
Anomalous Quantum Oscillations from Boson-Mediated Interband Scattering
L. Mangeolle, J. Knolle
Physical Review Letters 134 (14), 146502 (2025).
Quantum oscillations (QOs) in metals refer to the periodic variation of thermodynamic and transport properties as a function of inverse applied magnetic field. QO frequencies are normally associated with semiclassical trajectories of Fermi surface orbits, but recent experiments challenge the canonical description. We develop a theory of composite frequency quantum oscillations (CFQOs) in twodimensional Fermi liquids with several Fermi surfaces and interband scattering mediated by a dynamical boson, e.g., phonons or spin fluctuations. Specifically, we show that CFQOs arise from oscillations in the fermionic self-energy with anomalous frequency splitting and distinct strongly non-Lifshitz-Kosevich temperature dependences. Our theory goes beyond the framework of semiclassical Fermi surface trajectories highlighting the role of interaction effects. We provide experimental predictions and discuss the effect of nonequilibrium boson occupation in driven systems.
A Field Guide to Non-Onsager Quantum Oscillations in Metals
V. Leeb, N. Huber, C. Pfleiderer, J. Knolle, M. A. Wilde
Advanced Physics Research 4 (4), 2400134 (2025).
"Quantum oscillation (QO) measurements constitute a powerful method to measure the Fermi surface (FS) properties of metals. The observation of QOs is usually taken as strong evidence for the existence of extremal cross-sectional areas of the FS according to the famous Onsager relation. Here, mechanisms that generate QO frequencies that defy the Onsager relation are reviewed and material candidates are discussed. These include magnetic breakdown, magnetic interaction, chemical potential oscillations, and Stark quantum interference, most of which lead to signals occurring at combinations of ""parent"" Onsager frequencies. A special emphasis is put on the recently discovered mechanism of quasi-particle lifetime oscillations (QPLOs). This work aims to provide a field guide that allows, on the one hand, to distinguish such non-Onsager QOs from conventional QOs arising from extremal cross sections and, on the other hand, to distinguish the various non-Onsager mechanisms from each other. A practical classification of non-Onsager QOs is given in terms of the prerequisites for their occurrence and their characteristics. It is shown that, in particular, the recently discovered QPLOs may pose significant challenges for the interpretation of QO spectra, as they may occur quite generically as frequency differences in multi-orbit systems, without the necessity of visible ""parent"" frequencies in the spectrum, owing to a strongly suppressed temperature dephasing of QPLOs. An extensive list of material candidates is presented where QPLOs may represent an alternative explanation for the observation of unexpected QO frequencies."
Continuum of magnetic excitations in the Kitaev honeycomb iridate D3LiIr2O6
T. Halloran, Y. Wang, K. W. Plumb, M. B. Stone, B. Winn, M. K. Graves-Brook, J. A. Rodriguez-Rivera, Y. Qiu, P. Chauhan, J. Knolle, R. Moessner, N. P. Armitage, T. Takayama, H. Takagi, C. Broholm
Npj Quantum Materials 10 (1), 35 (2025).
Inelastic neutron scattering (INS) measurements of powder D-3(Li-7)(Ir-193)(2)O-6 reveal low energy magnetic excitations with a scattering cross-section that is broad in divided by Q divided by and energy transfer. The magnetic nature of the excitation spectrum is demonstrated by longitudinally polarized neutron scattering. The total magnetic moment of 1.8(4)mu(B)/Ir inferred from the observed magnetic scattering cross-section is consistent with the effective moment inferred from magnetic susceptibility data and expectations for the J(eff) = 1/2 single ion state. The rise in the dynamic correlation function S(Q, omega) for & hbar,.omega < 5 meV can be described by a simple model assuming nearest-neighbor anisotropic spin exchange, such as that found in the Kitaev model. Exchange disorder associated with the D site likely plays an important role in stabilizing the low T quantum fluctuating state.
Real-time scattering in the lattice Schwinger model
I. Papaefstathiou, J. Knolle, M. C. Banuls
Physical Review D 111 (2), 14504 (2025).
Tensor network methods have demonstrated their suitability for the study of equilibrium properties of lattice gauge theories, even close to the continuum limit. We use them in an out-of-equilibrium scenario, much less explored so far, by simulating the real-time collisions of composite mesons in the lattice Schwinger model. Constructing wave-packets of vector mesons at different incoming momenta, we observe the opening of the inelastic channel in which two heavier mesons are produced and identify the momentum threshold. To detect the products of the collision in the strong coupling regime we propose local quantitites that could be measured in current quantum simulation platforms.
Numerical study of quantum oscillations of quasiparticle lifetime: Impurity spectroscopy and electric field and strain effects
V. Leeb, J. Knolle
Physical Review B 110 (19), 195143 (2024).
Quantum oscillation (QO) measurements constitute one of the most powerful methods for determining the Fermi surface (FS) of metals, exploiting the famous Onsager relation between the FS area and the QO frequency. The recent observation of non-Onsager QOs with a frequency set by the difference of two FS orbits in a bulk three-dimensional metal can be understood as the QO of quasiparticle lifetime (QPL) due to interorbital scattering [N. Huber et al., Nature (London) 621, 276 (2023)]. QPL oscillations (QPLOs) generalize magnetointersubband oscillations known from coupled two-dimensional metals. They may provide a novel tool for extracting otherwise hard-to-measure intraband versus interband scattering times of quasiparticles. Here, we provide a numerical lattice study of QPLOs comparing transport and thermodynamic observables. We explore the effect of different imperfections like general impurities, Hall-effect-induced electric fields, various forms of strain from bending, and magnetic field inhomogeneities. We confirm the basic phenomenology of QPLOs as predicted in analytical calculations and identify additional nonperturbative features. Remarkably, we find that some imperfections can stabilize, or even enhance, non-Onsager QPLOs in contrast to standard QO frequencies. We discuss various avenues for identifying QPLOs in experiments and how to use their dependence on imperfections to extract material properties.
Spin-Peierls instability of the U(1) Dirac spin liquid (vol 15, 9577, 2024)
U. F. P. Seifert, J. Willsher, M. Drescher, F. Pollmann, J. Knolle
Nature Communications 15 (1), 9577 (2024).
Floquet prethermal order by disorder
H.-K. Jin, J. Knolle
Physical Review Research 6 (4), L042033 (2024).
Frustrated magnets can have accidental ground state degeneracies which may be lifted by various forms of disorder, for example in the form of thermal or quantum fluctuations. This order by disorder (ObD) paradigm is well established in equilibrium and here is generalized to Floquet many-body systems. Investigating a periodically driven XXZ-compass model on the square lattice, we show that in a prethermal regime, dynamical fluctuations induced by high-frequency drives select a discrete set of states out of a degenerate ground state manifold of the lowest order Floquet Hamiltonian chosen as initial states. Remarkably, prior to the ObD selection, an unusual fluctuating regime emerges leading to a prethermalization timescale scaling linearly with the drive frequency. We argue that prethermal ObD with its unusual approach to the selected states is a generic phenomenon of driven frustrated systems and confirm it in the paradigmatic J1-J2 XX model.
Interaction-Induced Crystalline Topology of Excitons
H. Davenport, J. Knolle, F. Schindler
Physical Review Letters 133 (17), 176601 (2024).
We apply the topological theory of symmetry indicators to interaction-induced exciton band structures in centrosymmetric semiconductors. Crucially, we distinguish between the topological invariants inherited from the underlying electron and hole bands and those that are intrinsic to the exciton wave function itself. Focusing on the latter, we show that there exists a class of exciton bands for which the maximally localized exciton Wannier states are shifted with respect to the electronic Wannier states by a quantized amount,. we call these excitons shift excitons. Our analysis explains how the exciton spectrum can be topologically nontrivial and sustain exciton edge states in open boundary conditions even when the underlying noninteracting bands have a trivial atomic limit. We demonstrate the presence of shift excitons as the lowest energy neutral excitations of the Su-Schrieffer-Heeger model in its trivial phase when supplemented by local two-body interactions.
Signatures of domain-wall confinement in Raman spectroscopy of Ising spin chains
S. Birnkammer, J. Knolle, M. Knap
Physical Review B 110 (13), 134408 (2024).
Mesonic bound states of domain walls (DWs) can be stabilized in quasi-one-dimensional magnetic compounds. Here, we theoretically study the Raman light scattering response of a twisted Kitaev chain with tilted magnetic fields as a minimal model for confinement in CoNb2O6. 2 O 6 . By both numerical matrix product states and few-DW variational states, we show that confinement-induced bound states directly manifest themselves as sharp peaks in the Raman response. Remarkably, by tuning the polarization of the incident light field, we demonstrate that the Raman response offers insights into the intrinsic symmetry of the bound-state wave function.
Spin-Peierls instability of deconfined quantum critical points
D. Hofmeier, J. Willsher, U. F. P. Seifert, J. Knolle
Physical Review B 110 (12), 125130 (2024).
Deconfined quantum critical points (DQCPs) are putative phase transitions beyond the Landau paradigm with emergent fractionalized degrees of freedom. The original example of a DQCP is the spin- 21 quantum antiferromagnet on the square lattice which features a second-order transition between valence bond solid (VBS) and N & eacute,.el order. The VBS order breaks a lattice symmetry, and the corresponding VBS order parameter may couple to lattice distortion modes (phonons) at appropriate momenta. We investigate a field-theoretic description of the DQCP in the presence of such a spin-lattice coupling. We show that treating phonons as classical lattice distortions leads to a relevant monopole-phonon interaction inducing an instability towards a distorted lattice by an analogous mechanism to the spin-Peierls instability in one dimension. Consequently, there is a breakdown of the DQCP which generally becomes a strong first-order transition. Taking into account the full quantum nature of the phonons, we argue that the continuous DQCP persists above a critical phonon frequency. Lastly, we comment on the connection to general gapless, deconfined gauge theories.
Kinetic ferromagnetism and topological magnons of the hole-doped Kitaev spin liquid
H.-K. Jin, W. Kadow, M. Knap, J. Knolle
Npj Quantum Materials 9 (1), 65 (2024).
We study the effect of hole doping on the Kitaev spin liquid (KSL) and find that for ferromagnetic (FM) Kitaev exchange K the system is very susceptible to the formation of a FM spin polarization. Through density matrix renormalization group simulations on finite systems, we uncover that the introduction of a single hole, corresponding to approximate to 1% hole doping for the system size we consider, with a hopping strength of just t similar to 0.28K is enough to disrupt fractionalization and polarize the spins in the [001] direction due to an order-by-disorder mechanism. Taking into account a material relevant FM anisotropic exchange Gamma drives the polarization towards the [111] direction via a transition into a topological FM state with chiral magnon excitations. We develop a parton mean-field theory incorporating fermionic holons and bosonic magnons, which accounts for the doping induced FM phases and topological magnon excitations. We discuss experimental implications for Kitaev candidate materials.
Spin-Peierls instability of the U(1) Dirac spin liquid
U. F. P. Seifert, J. Willsher, M. Drescher, F. Pollmann, J. Knolle
Nature Communications 15 (1), 7110 (2024).
Quantum fluctuations can inhibit long-range ordering in frustrated magnets and potentially lead to quantum spin liquid (QSL) phases. A prime example are gapless QSLs with emergent U(1) gauge fields, which have been understood to be described in terms of quantum electrodynamics in 2+1 dimension (QED3). Despite several promising candidate materials, however, a complicating factor for their realisation is the presence of other degrees of freedom. In particular lattice distortions can act to relieve magnetic frustration, precipitating conventionally ordered states. In this work, we use field-theoretic arguments as well as extensive numerical simulations to show that the U(1) Dirac QSL on the triangular and kagome lattices exhibits a weak-coupling instability due to the coupling of monopoles of the emergent gauge field to lattice distortions, leading to valence-bond solid ordering. This generalises the spin-Peierls instability of one-dimensional quantum critical spin chains to two-dimensional algebraic QSLs. We study static distortions as well as quantum-mechanical phonons. Even in regimes where the QSL is stable, the singular spin-lattice coupling leads to marked temperature-dependent corrections to the phonon spectrum, which provide salient experimental signatures of spin fractionalisation. We discuss the coupling of QSLs to the lattice as a general tool for their discovery and characterisation. Quantum spin liquids can emerge in frustrated magnets where quantum fluctuations prevent long-range order. Seifert et al. show that spin-lattice couplings can relieve magnetic frustration and destabilise 2D gapless quantum spin liquid states with fractionalised excitations, analogous to the 1D spin-Peierls instability.
Tunable band topology and optical conductivity in altermagnets
P. Rao, A. Mook, J. Knolle
Physical Review B 110 (2), 24425 (2024).
We study two-dimensional d-wave altermagnetic metals, taking into account the presence of substrate-induced Rashba spin-orbit coupling. We consider the altermagnet band structure using a 2D band Hamiltonian near the P point under external magnetic field. It is shown that time-reversal-symmetry breaking due to altermagnetism, together with Rashba coupling and external magnetic field, can result in nontrivial band topology. The topological phases can be tuned by magnetic field strength and directions, and are classified by their Chern numbers. Furthermore, we investigate the charge response by computing the full optical conductivity tensor with and without magnetic field. In particular, we focus on magneto-optical responses, which are the finite-frequency analog of the Berry curvature-induced anomalous Hall conductivity. Finally, using experimentally realistic parameters for RuO2, we estimate the Faraday angle in the absence of magnetic fields.
Realizing Altermagnetism in Fermi-Hubbard Models with Ultracold Atoms
P. Das, V. Leeb, J. Knolle, M. Knap
Physical Review Letters 132 (26), 263402 (2024).
Altermagnetism represents a type of collinear magnetism, that is in some aspects distinct from ferromagnetism and from conventional antiferromagnetism. In contrast to the latter, sublattices of opposite spin are related by spatial rotations and not only by translations and inversions. As a result, altermagnets have spin-split bands leading to unique experimental signatures. Here, we show theoretically how a d-wave altermagnetic phase can be realized with ultracold fermionic atoms in optical lattices. We propose an altermagnetic Hubbard model with anisotropic next-nearest neighbor hopping and obtain the Hartree-Fock phase diagram. The altermagnetic phase separates in a metallic and an insulating phase and is robust over a large parameter regime. We show that one of the defining characteristics of altermagnetism, the anisotropic spin transport, can be probed with trap-expansion experiments.
Spontaneous Formation of Altermagnetism from Orbital Ordering
V. Leeb, A. Mook, L. Smejkal, J. Knolle
Physical Review Letters 132 (23), 236701 (2024).
Altermagnetism has emerged as a third type of collinear magnetism. In contrast to standard ferromagnets and antiferromagnets, altermagnets exhibit extra even-parity wave spin order parameters resulting in a spin splitting of electronic bands in momentum space. In real space, sublattices of opposite spin polarization are anisotropic and related by rotational symmetry. In the hitherto identified altermagnetic candidate materials, the anisotropies arise from the local crystallographic symmetry. Here, we show that altermagnetism can also form as an interaction-induced electronic instability in a lattice without the crystallographic sublattice anisotropy. We provide a microscopic example of a two-orbital model showing that the coexistence of staggered antiferromagnetic and orbital order can realize robust altermagnetism. We quantify the spinsplitter conductivity as a key experimental observable and discuss material candidates for the interactioninduced realization of altermagnetism.
Neural Wave Functions for Superfluids
W. T. Lou, H. Sutterud, G. Cassella, W. M. C. Foulkes, J. Knolle, D. Pfau, J. S. Spencer
Physical Review X 14 (2), 21030 (2024).
Understanding superfluidity remains a major goal of condensed matter physics. Here, we tackle this challenge utilizing the recently developed fermionic neural network (FermiNet) wave function Ansatz [D. Pfau et al., Phys. Rev. Res. 2, 033429 (2020).] for variational Monte Carlo calculations. We study the unitary Fermi gas, a system with strong, short-range, two-body interactions known to possess a superfluid ground state but difficult to describe quantitatively. We demonstrate key limitations of the FermiNet Ansatz in studying the unitary Fermi gas and propose a simple modification based on the idea of an antisymmetric geminal power singlet (AGPs) wave function. The new AGPs FermiNet outperforms the original FermiNet significantly in paired systems, giving results which are more accurate than fixed-node diffusion Monte Carlo and are consistent with experiment. We prove mathematically that the new Ansatz, which differs from the original Ansatz only by the method of antisymmetrization, is a strict generalization of the original FermiNet architecture, despite the use of fewer parameters. Our approach shares several advantages with the original FermiNet: The use of a neural network removes the need for an underlying basis set,. sand the flexibility of the network yields extremely accurate results within a variational quantum Monte Carlo framework that provides access to unbiased estimates of arbitrary ground-state expectation values. We discuss how the method can be extended to study other superfluid.
Kitaev-Heisenberg model on the star lattice: From chiral Majorana fermions to chiral triplons
P. d'Ornellas, J. Knolle
Physical Review B 109 (9), 94421 (2024).
The interplay of frustrated interactions and lattice geometry can lead to a variety of exotic quantum phases. Here we unearth a particularly rich phase diagram of the Kitaev-Heisenberg model on the star lattice, a triangle decorated honeycomb lattice breaking sublattice symmetry. In the antiferromagnetic regime, the interplay of Heisenberg coupling and geometric frustration leads to the formation of valence bond solid (VBS) phases-a singlet VBS and a bond selective triplet VBS stabilized by the Kitaev exchange. We show that the ratio of the Kitaev versus Heisenberg exchange tunes between these VBS phases and chiral quantum spin-liquid regimes. Remarkably, the VBS phases host a whole variety of chiral triplon excitations with high Chern numbers in the presence of a weak magnetic field. We discuss our results in light of a recently synthesized star lattice material and other decorated lattice systems.
Quantum simulation of hadronic states with Rydberg-dressed atoms
Z. H. Wang, F. Y. Wang, J. Vovrosh, J. Knolle, F. Mintert, R. Mukherjee
Physical Review A 109 (3), 32613 (2024).
The phenomenon of confinement is well known in high-energy physics and can also be realized for low-energy domain-wall excitations in one-dimensional quantum spin chains. A bound state consisting of two domain walls can behave like a meson, and recently, Vovrosh et al. [PRX Quantum 3, 040309 (2022)] demonstrated that a pair of mesons could dynamically form a metastable confinement-induced bound state (consisting of four domain walls) akin to a hadronic state. However, the protocol discussed by Vovrosh et al. involving the use of interactions with characteristically nonmonotonic distance dependence is not easy to come by in nature, thus posing a challenge for its experimental realization. In this regard, Rydberg atoms can provide the required platform for simulating confinement-related physics. We exploit the flexibility offered by interacting Rydberg-dressed atoms to engineering modified spin-spin interactions for the one-dimensional transverse-field Ising model. Our numerical simulations show how Rydberg-dressed interactions can give rise to a variety of effective potentials that are suitable for hadron formation, which opens the possibility of simulating confinement physics with Rydberg platforms as a viable alternative to current trapped-ion experiments.
Single-hole spectra of Kitaev spin liquids: from dynamical Nagaoka ferromagnetism to spin-hole fractionalization
W. Kadow, H. K. Jin, J. Knolle, M. Knap
Npj Quantum Materials 9 (1), 32 (2024).
The dynamical response of a quantum spin liquid upon injecting a hole is a pertinent open question. In experiments, the hole spectral function, measured momentum-resolved in angle-resolved photoemission spectroscopy (ARPES) or locally in scanning tunneling microscopy (STM), can be used to identify spin liquid materials. In this study, we employ tensor network methods to simulate the time evolution of a single hole doped into the Kitaev spin-liquid ground state. Focusing on the gapped spin liquid phase, we reveal two fundamentally different scenarios. For ferromagnetic spin couplings, the spin liquid is highly susceptible to hole doping: a Nagaoka ferromagnet forms dynamically around the doped hole, even at weak coupling. By contrast, in the case of antiferromagnetic spin couplings, the hole spectrum demonstrates an intricate interplay between charge, spin, and flux degrees of freedom, best described by a parton mean-field ansatz of fractionalized holons and spinons. Moreover, we find a good agreement of our numerical results to the analytically solvable case of slow holes. Our results demonstrate that dynamical hole spectral functions provide rich information on the structure of fractionalized quantum spin liquids.
Interband scattering- and nematicity-induced quantum oscillation frequency in FeSe
V. Leeb, J. Knolle
Physical Review B 109 (8), L081109 (2024).
Understanding the nematic phase observed in the iron-chalcogenide materials is crucial for describing their superconducting pairing. Experiments on FeSe1-xSx showed that one of the slow Shubnikov-de Haas quantum oscillation frequencies disappears when tuning the material out of the nematic phase via chemical substitution or pressure, which has been interpreted as a Lifshitz transition [Coldea et al., npj Quantum Mater. 4, 2 (2019),. Reiss et al., Nat. Phys. 16, 89 (2020)]. Here, we present a generic, alternative scenario for a nematicity-induced sharp quantum oscillation frequency, which disappears in the tetragonal phase and is not connected to an underlying Fermi surface pocket. We show that different microscopic interband scattering mechanisms-for example, orbital-selective scattering-in conjunction with nematic order can give rise to this quantum oscillation frequency beyond the standard Onsager relation. We discuss implications for iron-chalcogenides and the interpretation of quantum oscillations in other correlated materials.
Quantum simulation of the one-dimensional Fermi-Hubbard model as a Z2 lattice-gauge theory
U. E. Khodaeva, D. L. Kovrizhin, J. Knolle
Physical Review Research 6 (1), 13032 (2024).
The Fermi-Hubbard model is one of the central paradigms in the physics of strongly correlated quantum many-body systems. Here we propose a quantum circuit algorithm based on the Z2 lattice gauge theory (LGT) representation of the one-dimensional Fermi-Hubbard model, which is suitable for implementation on current NISQ quantum computers. Within the LGT description there is an extensive number of local conserved quantities commuting with the Hamiltonian. We show how these conservation laws can be used to implement an efficient error-mitigation scheme. The latter is based on a postselection of states for noisy quantum simulators. While the LGT description requires a deeper quantum-circuit compared to a Jordan-Wigner (JW) based approach, remarkably, we find that our error-correction protocol leads to results being on par with a standard JW implementation on noisy quantum simulators.
Breakdown of chiral edge modes in topological magnon insulators
J. Habel, A. Mook, J. Willsher, J. Knolle
Physical Review B 109 (2), 24441 (2024).
Topological magnon insulators (TMI) are ordered magnets supporting chiral edge magnon excitations. These edge states are envisioned to serve as topologically protected information channels in low-loss magnonic devices. The standard description of TMI is based on linear spin-wave theory (LSWT), which approximates magnons as free noninteracting particles. However, magnon excitations of TMI are genuinely interacting even at zero temperature, calling into question descriptions based on LSWT alone. Here we perform a detailed nonlinear spin-wave analysis to investigate the stability of chiral edge magnons. We identify three general breakdown mechanisms: (1) The edge magnon couples to itself, generating a finite lifetime that can be large enough to lead to a spectral annihilation of the chiral state. (2) The edge magnon hybridizes with the extended bulk magnons and, as a consequence, delocalizes away from the edge. (3) Due to a bulk-magnon mediated edge-to-edge coupling, the chiral magnons at opposite edges hybridize. We argue that, in general, these breakdown mechanisms may invalidate predictions based on LSWT and violate the notion of topological protection. We discuss strategies how the breakdown of chiral edge magnons can be avoided, e.g., via the application of large magnetic fields. Our results highlight a challenge for the realization of chiral edge states in TMI and in other bosonic topological systems without particle number conservation.
Microscopic details of two-dimensional spectroscopy of one-dimensional quantum Ising magnets
G. Sim, F. Pollmann, J. Knolle
Physical Review B 108 (13), 134423 (2023).
The identification of microscopic systems describing the low-energy properties of correlated materials has been a central goal of spectroscopic measurements. We demonstrate how two-dimensional (2D) nonlinear spectroscopy can be used to distinguish effective spin systems whose linear responses show similar behavior. Motivated by recent experiments on the quasi-1D Ising magnet CoNb2O6, we focus on two proposed systems- the ferromagnetic twisted Kitaev spin chain with bond dependent interactions and the transverse field Ising chain. The dynamical spin structure factor probed in linear response displays similar broad spectra for both systems from their fermionic domain wall excitations. In sharp contrast, the 2D nonlinear spectra of the two systems show clear qualitative differences: those of the twisted Kitaev spin chain contain off-diagonal peaks originating from the bond dependent interactions and transitions between different fermion bands absent in the transverse field Ising chain. We discuss the different signatures of spin fractionalization in integrable and nonintegrable regimes of the systems and their connection to experiments.
An exact chiral amorphous spin liquid
G. Cassella, P. d'Ornellas, T. Hodson, W. M. H. Natori, J. Knolle
Nature Communications 14 (1), 6663 (2023).
Topological insulator phases of non-interacting particles have been generalized from periodic crystals to amorphous lattices, which raises the question whether topologically ordered quantum many-body phases may similarly exist in amorphous systems? Here we construct a soluble chiral amorphous quantum spin liquid by extending the Kitaev honeycomb model to random lattices with fixed coordination number three. The model retains its exact solubility but the presence of plaquettes with an odd number of sides leads to a spontaneous breaking of time reversal symmetry. We unearth a rich phase diagram displaying Abelian as well as a non-Abelian quantum spin liquid phases with a remarkably simple ground state flux pattern. Furthermore, we show that the system undergoes a finite-temperature phase transition to a conducting thermal metal state and discuss possible experimental realisations. Recently topological phases have been generalized to amorphous materials, but demonstrations have been limited to non-interacting particles. Cassella et al. show the emergence of chiral amorphous quantum spin liquid in an exactly soluble model by extending the Kitaev honeycomb model to random lattices.
Quantum oscillations of the quasiparticle lifetime in a metal
N. Huber, V. Leeb, A. Bauer, G. Benka, J. Knolle, C. Pfleiderer, M. A. Wilde
Nature 621 (7978), 276-+ (2023).
Following nearly a century of research, it remains a puzzle that the low-lying excitations of metals are remarkably well explained by effective single-particle theories of non-interacting bands(1-4). The abundance of interactions in real materials raises the question of direct spectroscopic signatures of phenomena beyond effective single-particle, single-band behaviour. Here we report the identification of quantum oscillations (QOs) in the three-dimensional topological semimetal CoSi, which defy the standard description in two fundamental aspects. First, the oscillation frequency corresponds to the difference of semiclassical quasiparticle (QP) orbits of two bands, which are forbidden as half of the trajectory would oppose the Lorentz force. Second, the oscillations exist up to above 50 K, in strong contrast to all other oscillatory components, which vanish below a few kelvin. Our findings are in excellent agreement with generic model calculations of QOs of the QP lifetime (QPL). Because the only precondition for their existence is a nonlinear coupling of at least two electronic orbits, for example, owing to QP scattering on defects or collective excitations, such QOs of the QPL are generic for any metal featuring Landau quantization with several orbits. They are consistent with certain frequencies in topological semimetals(5-9), unconventional superconductors(10,11), rare-earth compounds(12-14) and Rashba systems(15), and permit to identify and gauge correlation phenomena, for example, in two-dimensional materials(16,17) and multiband metals(18).
Temporal disorder in spatiotemporal order
H. Z. Zhao, J. Knolle, R. Moessner
Physical Review B 108 (10), L100203 (2023).
Time-dependent driving holds the promise of realizing dynamical phenomena absent in static systems. Here, we introduce a correlated random driving protocol to realize a spatiotemporal order that cannot be achieved even by periodic driving, thereby extending the discussion of time translation symmetry breaking to randomly driven systems. We find a combination of temporally disordered micromotion with prethermal stroboscopic spatiotemporal long-range order. This spatiotemporal order remains robust against generic perturbations, with an algebraically long prethermal lifetime where the scaling exponent strongly depends on the symmetry of the perturbation, which we account for analytically.
Quantum liquids of the S=3/2 Kitaev honeycomb and related Kugel-Khomskii models
W. M. H. Natori, H. K. Jin, J. Knolle
Physical Review B 108 (7), (2023).
Theory of difference-frequency quantum oscillations
V. Leeb, J. Knolle
Physical Review B 108 (5), 54202 (2023).
Quantum oscillations (QOs) describe the periodic variation of physical observables as a function of inverse magnetic field in metals. The Onsager relation connects the basic QO frequencies with the extremal areas of closed Fermi surface pockets, and the theory of magnetic breakdown explains the observation of sums of QO frequencies at high magnetic fields. Here we develop a quantitative theory of difference-frequency QOs in two and three-dimensional metals with multiple Fermi pockets with parabolic or linearly dispersing excitations. We show that a nonlinear interband coupling, e.g., in the form of interband impurity scattering, can give rise to otherwise forbidden QO frequencies which can persist to much higher temperatures compared to the basis frequencies. We discuss the experimental implications of our findings for various material candidates, for example multifold fermion systems, like CoSi, and the relation to magneto-intersubband oscillations known for coupled two-dimensional electron gases.
Fractionalized Prethermalization in a Driven Quantum Spin Liquid
H. K. Jin, J. Knolle, M. Knap
Physical Review Letters 130 (22), 226701 (2023).
Quantum spin liquids subject to a periodic drive can display fascinating nonequilibrium heating behavior because of their emergent fractionalized quasiparticles. Here, we investigate a driven Kitaev honeycomb model and examine the dynamics of emergent Majorana matter and Z2 flux excitations. We uncover a distinct two-step heating profile-dubbed fractionalized prethermalization-and a quasistationary state with vastly different temperatures for the matter and the flux sectors. We argue that this peculiar prethermalization behavior is a consequence of fractionalization. Furthermore, we discuss an exper-imentally feasible protocol for preparing a zero-flux initial state of the Kiteav honeycomb model with a low energy density, which can be used to observe fractionalized prethermalization in quantum information processing platforms.
Twisting the Dirac cones of the SU(4) spin-orbital liquid on the honeycomb lattice
H. K. Jin, W. M. H. Natori, J. Knolle
Physical Review B 107 (18), L180401 (2023).
By combining the density matrix renormalization group (DMRG) method with Gutzwiller projected wave functions, we study the SU(4) symmetric spin-orbital model on the honeycomb lattice. We find that the ground states can be well described by a Gutzwiller projected pi-flux state with Dirac-type gapless excitations at one quarter filling. Although these Dirac points are gapped by emergent gauge fluxes on finite cylinders, they govern the critical behavior in the thermodynamic limit. By inserting a theta = pi spin flux to twist the boundary condition, we can shift the gapless sector to the ground state, which provides compelling evidence for the presence of a gapless Dirac spin-orbital liquid.
Nonlinear spectroscopy of bound states in perturbed Ising spin chains
G. Sim, J. Knolle, F. Pollmann
Physical Review B 107 (10), L100404 (2023).
We study the nonlinear response of nonintegrable one-dimensional (1D) spin models using infinite matrix-product state techniques. As a benchmark and demonstration of the method, we first calculate the two-dimensional (2D) coherent spectroscopy for the exactly soluble ferromagnetic transverse field Ising model where excitations are freely moving domain walls. We then investigate the distinct signatures of confined bound states by introducing a longitudinal field and observe the emergence of strong nonrephasinglike signals. To interpret the observed phenomena, we use a two-kink approximation to perturbatively compute the 2D spectra. We find good agreement in comparison with the exact results of the infinite matrix-product state method in the strongly confined regime. We discuss the relevance of our results for quasi-1D Ising spin chain materials, such as CoNb2O6.
Magnetic excitations, phase diagram, and order-by-disorder in the extended triangular-lattice Hubbard model
J. Willsher, H. K. Jin, J. Knolle
Physical Review B 107 (6), 64425 (2023).
The dynamical structure factor is an important observable of quantum magnets but due to numerical and theoretical limitations, it remains a challenge to make predictions for Hubbard-like models beyond one di-mension. In this work, we study the magnetic excitations of the triangular lattice Hubbard model including next-nearest-neighbor hopping. Starting from the expected 120 degrees and stripe magnetic orders, we compute the magnon spectra within a self-consistent random phase approximation. In the stripe phase, we generically find accidental zero modes related to a classical degeneracy known from the corresponding J1 -J2 Heisenberg model. We extend the order-by-disorder mechanism to Hubbard systems and show how quantum fluctuations stabilize the stripe order. In addition, the frustration-induced condensation of magnon modes allows us to map out the entire phase diagram which is in remarkable agreement with recent numerical works. We discuss connections to experiments on triangular lattice compounds and the relation of our results to the proposed chiral spin liquid phase.
Bridging the gap between classical and quantum many-body information dynamics
A. Pizzi, D. Malz, A. Nunnenkamp, J. Knolle
Physical Review B 106 (21), 214303 (2022).
"The fundamental question of how information spreads in closed quantum many-body systems is often addressed through the lens of the bipartite entanglement entropy, a quantity that describes correlations in a comprehensive (nonlocal) way. Among the most striking features of the entanglement entropy are its unbounded linear growth in the thermodynamic limit, its asymptotic extensivity in finite-size systems, and the possibility of measurement-induced phase transitions, all of which have no obvious classical counterpart. Here, we show how these key qualitative features emerge naturally also in classical information spreading, as long as one treats the classical many-body problem on par with the quantum one, that is, by explicitly accounting for the exponentially large classical probability distribution. Our analysis is supported by extensive numerics on prototypical cellular automata and Hamiltonian systems, for which we focus on the classical mutual information and also introduce a ""classical entanglement entropy."" Our study sheds light on the nature of information spreading in classical and quantum systems, and opens avenues for quantum-inspired classical approaches across physics, information theory, and statistics."
Thermal spin dynamics of Kitaev magnets: Scattering continua and magnetic field induced phases within a stochastic semiclassical approach
O. Franke, D. Calugaru, A. Nunnenkamp, J. Knolle
Physical Review B 106 (17), 174428 (2022).
"The honeycomb magnet a-RuCl3 is a prime candidate material for realizing the Kitaev quantum spin liquid (QSL), but it shows long-range magnetic order at low temperature. Nevertheless, its broad inelastic neutron scattering (INS) response at finite frequency has been interpreted as that of a ""proximate QSL."" A moderate in-plane magnetic field indeed melts the residual zigzag order, giving rise to peculiar intermediate-field phases before the high-field polarized state. In INS measurements the low-frequency spin waves disappear, leading to a broad scattering continuum in the field-induced intermediate regime, whose nature is currently under debate. Here, we study the magnetic-field-dependent spin dynamics of the K -F -F' model within a stochastic semiclassical treatment, which incorporates the effect of finite-temperature fluctuations. At temperatures relevant for INS experiments, we show how the excitations of the zigzag phase broaden and that the different intermediate phases all show a similar continuum response. We discuss the implications of our results for experiments and highlight the importance of distinguishing finite-temperature fluctuations from genuine quantum fractionaliza-tion signatures in frustrated magnets."
Disorder-free localization with Stark gauge protection
H. F. Lang, P. Hauke, J. Knolle, F. Grusdt, J. C. Halimeh
Physical Review B 106 (17), 174305 (2022).
Disorder-free localization in translation-invariant gauge theories presents a counterintuitive yet powerful framework of ergodicity breaking in quantum many-body physics. The fragility of this phenomenon in the presence of gauge-breaking errors has recently been addressed, but no scheme has been able to reliably stabilize disorder-free localization through all accessible evolution times while preserving the disorder-free property. Here, we introduce the concept of Stark gauge protection, which entails a linear sum in gauge-symmetry local (pseudo)generators weighted by a Stark potential. Using exact diagonalization and Krylov-based methods, we show how this scheme can stabilize or even enhance disorder-free localization against gauge-breaking errors in U(1) and Z2 gauge theories up to all accessible evolution times, without inducing bona fide Stark many-body localization. We show through a Magnus expansion that the dynamics under Stark gauge protection is described by an effective Hamiltonian where gauge-breaking terms are suppressed locally by the protection strength and additionally by the matter site index, which we argue is the main reason behind stabilizing the localization up to all accessible times. Our scheme is readily feasible in modern ultracold-atom experiments and Rydberg-atom setups with optical tweezers.
Prethermal nematic order and staircase heating in a driven frustrated Ising magnet with dipolar interactions
H. K. Jin, A. Pizzi, J. Knolle
Physical Review B 106 (14), 144312 (2022).
Many-body systems subject to a high-frequency drive can show intriguing thermalization behavior. Prior to heating to a featureless infinite-temperature state, these systems can spend an exponentially long time in prethermal phases characterized by various kinds of order. Here, we uncover the rich nonequilibrium phase diagram of a driven frustrated two-dimensional Ising magnet with competing short-range ferromagnetic and long-range dipolar interactions. We show that the ordered stripe and nematic phases, which appear in equilibrium as a function of temperature, underpin subsequent prethermal phases in a new multistep heating process en route towards the ultimate heat death. We discuss implications for experiments on ferromagnetic thin films and other driving induced phenomena in frustrated magnets.
Dynamical Hadron Formation in Long-Range Interacting Quantum Spin Chains
J. Vovrosh, R. Mukherjee, A. Bastianello, J. Knolle
Prx Quantum 3 (4), 40309 (2022).
The study of confinement in quantum spin chains has seen a large surge of interest in recent years. It is not only important for understanding a range of effective one-dimensional condensed-matter realiza-tions but it also shares some of the nonperturbative physics with quantum chromodynamics (QCD), which makes it a prime target for current quantum simulation efforts. In analogy to QCD, the confinement -induced two-particle bound states that appear in these models are dubbed mesons. Here, we study scattering events due to meson collisions in a quantum spin chain with long-range interactions such that two mesons have an extended interaction. We show how novel hadronic bound states, e.g., with four con-stituent particles akin to tetraquarks, may form dynamically in fusion events. In a natural collision their signal is weak, as elastic meson scattering dominates. However, we propose two controllable protocols that allow for a clear observation of dynamical hadron formation. We discuss how this physics can be simulated in trapped-ion or Rydberg-atom setups.
Suppression of Interband Heating for Random Driving
H. Z. Zhao, J. Knolle, R. Moessner, F. Mintert
Physical Review Letters 129 (12), 120605 (2022).
Heating to high-lying states strongly limits the experimental observation of driving induced non -equilibrium phenomena, particularly when the drive has a broad spectrum. Here we show that, for entire families of structured random drives known as random multipolar drives, particle excitation to higher bands can be well controlled even away from a high-frequency driving regime. This opens a window for observing drive-induced phenomena in a long-lived prethermal regime in the lowest band.
Unveiling the S=3/2 Kitaev honeycomb spin liquids
H. K. Jin, W. M. H. Natori, F. Pollmann, J. Knolle
Nature Communications 13 (1), 3813 (2022).
Recently, material realizations of the spin 3/2 Kitaev honeycomb model have been proposed, but the model has not been solved by either analytical or numerical methods. Here the authors report exact results for the spin 3/2 model consistent with numerical simulations, and find gapped and gapless quantum spin liquids. The S=3/2 Kitaev honeycomb model (KHM) is a quantum spin liquid (QSL) state coupled to a static Z(2) gauge field. Employing an SO(6) Majorana representation of spin3/2's, we find an exact representation of the conserved plaquette fluxes in terms of static Z(2) gauge fields akin to the S=1/2 KHM which enables us to treat the remaining interacting matter fermion sector in a parton mean-field theory. We uncover a ground-state phase diagram consisting of gapped and gapless QSLs. Our parton description is in quantitative agreement with numerical simulations, and is furthermore corroborated by the addition of a [001] single ion anisotropy (SIA) which continuously connects the gapless Dirac QSL of our model with that of the S=1/2 KHM. In the presence of a weak [111] SIA, we discuss an emergent chiral QSL within a perturbation theory.
Measurement-induced phase transition in a chaotic classical many-body system
J. Willsher, S. W. Liu, R. Moessner, J. Knolle
Physical Review B 106 (2), 24305 (2022).
Local measurements in quantum systems are projective operations which act to counteract the spread of quan-tum entanglement. Recent work has shown that local, random measurements applied to a generic volume-law entanglement generating many-body system are able to force a transition into an area-law phase. This work shows that projective operations can also force a similar classical phase transition,. we show that local projections in a chaotic system can freeze information dynamics. In rough analogy with measurement-induced phase transitions, this is characterized by an absence of information spreading instead of entanglement entropy. We leverage a damage-spreading model of the classical transition to predict the butterfly velocity of the system both near to and away from the transition point. We map out the full phase diagram and show that the critical point is shifted by local projections, but remains in the directed percolation universality class. We discuss the implication for other classical chaotic many-body systems and the relation to synchronization transitions.
Berry curvature-induced local spin polarisation in gated graphene/WTe2 heterostructures
L. Powalla, J. Kiemle, E. J. Konig, A. P. Schnyder, J. Knolle, K. Kern, A. Holleitner, C. Kastl, M. Burghard
Nature Communications 13 (1), 3152 (2022).
Experimental control of local spin-charge interconversion is of primary interest for spintronics. Van der Waals (vdW) heterostructures combining graphene with a strongly spin-orbit coupled two-dimensional (2D) material enable such functionality by design. Electric spin valve experiments have thus far provided global information on such devices, while leaving the local interplay between symmetry breaking, charge flow across the heterointerface and aspects of topology unexplored. Here, we probe the gate-tunable local spin polarisation in current-driven graphene/WTe2 heterostructures through magneto-optical Kerr microscopy. Even for a nominal in-plane transport, substantial out-of-plane spin accumulation is induced by a corresponding out-of-plane current flow. We present a theoretical model which fully explains the gate- and bias-dependent onset and spatial distribution of the intense Kerr signal as a result of a non-linear anomalous Hall effect in the heterostructure, which is enabled by its reduced point group symmetry. Our findings unravel the potential of 2D heterostructure engineering for harnessing topological phenomena for spintronics, and constitute an important step toward nanoscale, electrical spin control. Spin-based electronics offers significantly improved efficiency, but a major challenge is the electric manipulation of spin. Here, Powalla et al find a large gate induced spinpolarization in graphene/WTe2 heterostructures, illustrating the potential of such heterostructures for spintronics.
Localization persisting under aperiodic driving
H. Z. Zhao, F. Mintert, J. Knolle, R. Moessner
Physical Review B 105 (22), L220202 (2022).
"Localization may survive in periodically driven (Floquet) quantum systems, but is generally unstable for aperiodic drives. In this Letter, we identify a hidden conservation law originating from a chiral symmetry in a disordered spin-21 XX chain. This protects indefinitely long-lived localization for general-even aperiodic-drives. Therefore, rather counterintuitively, adding further potential disorder which spoils the conservation law delocalizes the system, via a controllable parametrically long-lived prethermal regime. This provides an example of persistent single-particle ""localization without eigenstates."""
Anomalous random multipolar driven insulators
H. Z. Zhao, M. S. Rudner, R. Moessner, J. Knolle
Physical Review B 105 (24), 245119 (2022).
It is by now well established that periodically driven quantum many-body systems can realize topological nonequilibrium phases without any equilibrium counterpart. Here we show that, even in the absence of time translation symmetry, nonequilibrium topological phases of matter can exist in aperiodically driven systems for tunably parametrically long prethermal lifetimes. As a prerequisite, we first demonstrate the existence of longlived prethermal Anderson localization in two dimensions under random multipolar driving. We then show that the localization may be topologically nontrivial with a quantized bulk orbital magnetization even though there are no well-defined Floquet operators. We further confirm the existence of this anomalous random multipolar driven insulator by detecting quantized charge pumping at the boundaries, which renders it experimentally observable.
Enhancing Disorder-Free Localization through Dynamically Emergent Local Symmetries
J. C. Halimeh, L. Homeier, H. Z. Zhao, A. Bohrdt, F. Grusdt, P. Hauke, J. Knolle
Prx Quantum 3 (2), 19 (2022).
Disorder-free localization is a recently discovered phenomenon of nonergodicity that can emerge in quantum many-body systems hosting gauge symmetries when the initial state is prepared in a superposition of gauge superselection sectors. Thermalization is then prevented up to all accessible evolution times despite the model being nonintegrable and translation invariant. In a recent work [Halimeh et al., arXiv:2111.02427 (2021)], it has been shown that terms linear in the gauge-symmetry generator stabilize disorder-free localization in U(1) gauge theories against gauge errors that couple different superselection sectors. Here, we show in the case of Z2 gauge theories that disorder-free localization can not only be stabilized, but also enhanced by the addition of translation-invariant terms linear in a local Z2 pseudogenerator that acts identically to the full generator in a single superselection sector, but not necessarily outside of it. We show analytically and numerically how this leads through the quantum Zeno effect to the dynamical emergence of a renormalized gauge theory with an enhanced local symmetry, which contains the Z2 gauge symmetry of the ideal model, associated with the Z2 pseudogenerator. The resulting proliferation of superselection sectors due to this dynamically emergent gauge theory creates an effective disorder greater than that in the original model, thereby enhancing disorder-free localization. We demonstrate the experimental feasibility of the Z2 pseudogenerator by providing a detailed readily implementable experimental proposal for the observation of disorder-free localization in a Rydberg setup.
Optical phonons coupled to a Kitaev spin liquid
A. Metavitsiadis, W. Natori, J. Knolle, W. Brenig
Physical Review B 105 (16), 165151 (2022).
Emergent excitation continua in frustrated magnets are a fingerprint of fractionalization, characteristic of quantum spin-liquid states. Recent evidence from Raman scattering for a coupling between such continua and lattice degrees of freedom in putative Kitaev magnets may provide insight into the nature of the fractionalized quasiparticles. Here we study the renormalization of optical phonons coupled to the underlying Z2 quantum spin liquid. We show that phonon line shapes acquire an asymmetry, observable in light scattering and originating from two distinct sources, namely, the dispersion of the Majorana continuum and the Fano effect. Moreover, we find that the phonon lifetimes increase with increasing temperature due to thermal blocking of the available phase space. Finally, in contrast to low-energy probes, optical phonon renormalization is rather insensitive to thermally excited gauge fluxes and barely susceptible to external magnetic fields.
Confinement-induced impurity states in spin chains
J. Vovrosh, H. Z. Zhao, J. Knolle, A. Bastianello
Physical Review B 105 (10), L100301 (2022).
Quantum simulators hold the promise of probing central questions of high-energy physics in tunable condensed matter platforms, for instance, the physics of confinement. Local defects can be an obstacle in these setups, harming their simulation capabilities. However, defects in the form of impurities can also be useful as probes of many-body correlations and may lead to fascinating new phenomena themselves. Here, we investigate the interplay between impurity and confinement physics in a basic spin chain setup, showing the emergence of exotic excitations as impurity-meson bound states with a long lifetime. For weak confinement, semiclassical approximations can describe the capture process in a meson-impurity scattering event. In the strong-confining regime, intrinsic quantum effects are visible through the quantization of the emergent bound state energies which can be in simulators.
Orthogonal Quantum Many-Body Scars
H. Z. Zhao, A. Smith, F. Mintert, J. Knolle
Physical Review Letters 127 (15), 150601 (2021).
Quantum many-body scars have been put forward as counterexamples to the eigenstate thermalization hypothesis. These atypical states are observed in a range of correlated models as long-lived oscillations of local observables in quench experiments starting from selected initial states. The long-time memory is a manifestation of quantum nonergodicity generally linked to a subextensive generation of entanglement entropy, the latter of which is widely used as a diagnostic for identifying quantum many-body scars numerically as low entanglement outliers. Here we show that by adding kinetic constraints to a fractionalized orthogonal metal, we can construct a minimal model with orthogonal quantum many-body scars leading to persistent oscillations with infinite lifetime coexisting with rapid volume-law entanglement generation. Our example provides new insights into the link between quantum ergodicity and many-body entanglement while opening new avenues for exotic nonequilibrium dynamics in strongly correlated multicomponent quantum systems.
Classical approaches to prethermal discrete time crystals in one, two, and three dimensions
A. Pizzi, A. Nunnenkamp, J. Knolle
Physical Review B 104 (9), 94308 (2021).
We provide a comprehensive account of prethermal discrete time crystals within classical Hamiltonian dynamics, complementing and extending our recent work [A. Pizzi, A. Nunnenkamp, and J. Knolle, Phys. Rev. Lett. 127, 140602 (2021)]. Considering power-law interacting spins on one-, two-, and three-dimensional hypercubic lattices, we investigate the interplay between dimensionality and interaction range in the stabilization of these nonequilibrium phases of matter that break the discrete time-translational symmetry of a periodic drive.
Simple mitigation of global depolarizing errors in quantum simulations
J. Vovrosh, K. E. Khosla, S. Greenaway, C. Self, M. S. Kim, J. Knolle
Physical Review E 104 (3), 35309 (2021).
To get the best possible results from current quantum devices error mitigation is essential. In this work we present a simple but effective error mitigation technique based on the assumption that noise in a deep quantum circuit is well described by global depolarizing error channels. By measuring the errors directly on the device, we use an error model ansatz to infer error-free results from noisy data. We highlight the effectiveness of our mitigation via two examples of recent interest in quantum many-body physics: entanglement measurements and real-time dynamics of confinement in quantum spin chains. Our technique enables us to get quantitative results from the IBM quantum computers showing signatures of confinement, i.e., we are able to extract the meson masses of the confined excitations which were previously out of reach. Additionally, we show the applicability of this mitigation protocol in a wider setting with numerical simulations of more general tasks using a realistic error model. Our protocol is device-independent, simply implementable, and leads to large improvements in results if the global errors are well described by depolarization.
Classical Prethermal Phases of Matter
A. Pizzi, A. Nunnenkamp, J. Knolle
Physical Review Letters 127 (14), 140602 (2021).
Systems subject to a high-frequency drive can spend an exponentially long time in a prethermal regime, in which novel phases of matter with no equilibrium counterpart can be realized. Because of the notorious computational challenges of quantum many-body systems, numerical investigations in this direction have remained limited to one spatial dimension, in which long-range interactions have been proven a necessity. Here, we show that prethermal nonequilibrium phases of matter are not restricted to the quantum domain. Studying the Hamiltonian dynamics of a large three-dimensional lattice of classical spins, we provide the first numerical proof of prethermal phases of matter in a system with short-range interactions. Concretely, we find higher-order as well as fractional discrete time crystals breaking the time-translational symmetry of the drive with unexpectedly large integer as well as fractional periods. Our work paves the way toward the exploration of novel prethermal phenomena by means of classical Hamiltonian dynamics with virtually no limitations on the system's geometry or size, and thus with direct implications for experiments.
Variational quantum algorithm with information sharing
C. N. Self, K. E. Khosla, A. W. R. Smith, F. Sauvage, P. D. Haynes, J. Knolle, F. Mintert, M. S. Kim
Npj Quantum Information 7 (1), 116 (2021).
We introduce an optimisation method for variational quantum algorithms and experimentally demonstrate a 100-fold improvement in efficiency compared to naive implementations. The effectiveness of our approach is shown by obtaining multi-dimensional energy surfaces for small molecules and a spin model. Our method solves related variational problems in parallel by exploiting the global nature of Bayesian optimisation and sharing information between different optimisers. Parallelisation makes our method ideally suited to the next generation of variational problems with many physical degrees of freedom. This addresses a key challenge in scaling-up quantum algorithms towards demonstrating quantum advantage for problems of real-world interest.
Rigorous Bounds on the Heating Rate in Thue-Morse Quasiperiodically and Randomly Driven Quantum Many-Body Systems
T. Mori, H. Z. Zhao, F. Mintert, J. Knolle, R. Moessner
Physical Review Letters 127 (5), 50602 (2021).
The nonequilibrium quantum dynamics of closed many-body systems is a rich yet challenging field. While recent progress for periodically driven (Floquet) systems has yielded a number of rigorous results, our understanding on quantum many-body systems driven by rapidly varying but aperiodic and quasiperiodic driving is still limited. Here, we derive rigorous, nonperturbative, bounds on the heating rate in quantum many-body systems under Thue-Morse quasiperiodic driving and under random multipolar driving, the latter being a tunably randomized variant of the former. In the process, we derive a static effective Hamiltonian that describes the transient prethermal state, including the dynamics of local observables. Our bound for Thue-Morse quasiperiodic driving suggests that the heating time scales like (omega/g)(-C) (ln()(omega/)(g)) with a positive constant C and a typical energy scale g of the Hamiltonian, in agreement with our numerical simulations.
One-dimensional long-range Falikov-Kimball model: Thermal phase transition and disorder-free localization
T. Hodson, J. Willsher, J. Knolle
Physical Review B 104 (4), 45116 (2021).
Disorder or interactions can turn metals into insulators. One of the simplest settings in which to study this physics is given by the Falikov-Kimball (FK) model, which describes itinerant fermions interacting with a classical Ising background field. Despite the translational invariance of the model, inhomogeneous configurations of the background field give rise to effective disorder physics which lead to a rich phase diagram in two (or more) dimensions with finite-temperature charge-density wave (CDW) transitions and interaction-tuned Anderson versus Mott localized phases. Here, we propose a generalized FK model in one dimension with long-range interactions which shows a similarly rich phase diagram. We use an exact Markov chain Monte Carlo method to map the phase diagram and compute the energy-resolved localization properties of the fermions. We compare the behavior of this transitionally invariant model to an Anderson model of uncorrelated binary disorder about a background CDW field which confirms that the fermionic sector only fully localizes for very large system sizes.
Flat and correlated plasmon bands in graphenek/alpha-RuCl3 heterostructures
H. K. Jin, J. Knolle
Physical Review B 104 (4), 45140 (2021).
We develop a microscopic theory for plasmon excitations of graphene/alpha-RuCl3 heterostructures. Within a Kondo-Kitaev model with various interactions, a heavy Fermi liquid hosting flat bands emerges in which the itinerant electrons of graphene effectively hybridize with the fractionalized fermions of the Kitaev quantum spin liquid. We find novel correlated plasmon bands induced by the interplay of flat bands and interactions and argue that our theory is consistent with the available experimental data on graphene/alpha-RuCl3 heterostructures. We predict novel plasmon branches beyond the long-wavelength limit and discuss the implications for probing correlation phenomena in other flat band systems.
Confinement and entanglement dynamics on a digital quantum computer
J. Vovrosh, J. Knolle
Scientific Reports 11 (1), 11577 (2021).
Confinement describes the phenomenon when the attraction between two particles grows with their distance, most prominently found in quantum chromodynamics (QCD) between quarks. In condensed matter physics, confinement can appear in quantum spin chains, for example, in the one dimensional transverse field Ising model (TFIM) with an additional longitudinal field, famously observed in the quantum material cobalt niobate or in optical lattices. Here, we establish that state-of-the-art quantum computers have reached capabilities to simulate confinement physics in spin chains. We report quantitative confinement signatures of the TFIM on an IBM quantum computer observed via two distinct velocities for information propagation from domain walls and their mesonic bound states. We also find the confinement induced slow down of entanglement spreading by implementing randomized measurement protocols for the second order Renyi entanglement entropy. Our results are a crucial step for probing non-perturbative interacting quantum phenomena on digital quantum computers beyond the capabilities of classical hardware.
Higher-order and fractional discrete time crystals in clean long-range interacting systems
A. Pizzi, J. Knolle, A. Nunnenkamp
Nature Communications 12 (1), 2341 (2021).
Discrete time crystals are periodically driven systems characterized by a response with periodicity nT, with T the period of the drive and n>1. Typically, n is an integer and bounded from above by the dimension of the local (or single particle) Hilbert space, the most prominent example being spin-1/2 systems with n restricted to 2. Here, we show that a clean spin-1/2 system in the presence of long-range interactions and transverse field can sustain a huge variety of different 'higher-order' discrete time crystals with integer and, surprisingly, even fractional n>2. We characterize these (arguably prethermal) non-equilibrium phases of matter thoroughly using a combination of exact diagonalization, semiclassical methods, and spin-wave approximations, which enable us to establish their stability in the presence of competing long- and short-range interactions. Remarkably, these phases emerge in a model with continous driving and time-independent interactions, convenient for experimental implementations with ultracold atoms or trapped ions.
Gapless state of interacting Majorana fermions in a strain-induced Landau level
A. Agarwala, S. Bhattacharjee, J. Knolle, R. Moessner
Physical Review B 103 (13), 134427 (2021).
Mechanical strain can generate a pseudomagnetic field, and hence Landau levels (LL), for low-energy excitations of quantum matter in two dimensions. We study the collective state of the fractionalized Majorana fermions arising from residual generic spin interactions in the central LL, where the projected Hamiltonian reflects the spin symmetries in intricate ways: emergent U(1) and particle-hole symmetries forbid any bilinear couplings, leading to an intrinsically strongly interacting system,. also, they allow the definition of a filling fraction, which is fixed at 1/2. We argue that the resulting many-body state is gapless within our numerical accuracy, implying ultra-short-ranged spin correlations, while chirality correlators decay algebraically. This amounts to a Kitaev 'non-Fermi' spin liquid and shows that interacting Majorana Fermions can exhibit intricate behavior akin to fractional quantum Hall physics in an insulating magnet.
Anomalous Quantum Oscillations in a Heterostructure of Graphene on a Proximate Quantum Spin Liquid
V. Leeb, K. Polyudov, S. Mashhadi, S. Biswas, R. Valenti, M. Burghard, J. Knolle
Physical Review Letters 126 (9), 97201 (2021).
The quasi-two-dimensional Mott insulator alpha-RuCl3 is proximate to the sought-after Kitaev quantum spin liquid (QSL). In a layer of alpha-RuCl3 on graphene, the dominant Kitaev exchange is further enhanced by strain. Recently, quantum oscillation (QO) measurements of such alpha-RuCl3 and graphene heterostructures showed an anomalous temperature dependence beyond the standard Lifshitz-Kosevich (LK) description. Here, we develop a theory of anomalous QO in an effective Kitaev-Kondo lattice model in which the itinerant electrons of the graphene layer interact with the correlated magnetic layer via spin interactions. At low temperatures, a heavy Fermi liquid emerges such that the neutral Majorana fermion excitations of the Kitaev QSL acquire charge by hybridizing with the graphene Dirac band. Using ab initio calculations to determine the parameters of our low-energy model, we provide a microscopic theory of anomalous QOs with a non-LK temperature dependence consistent with our measurements. We show how remnants of fractionalized spin excitations can give rise to characteristic signatures in QO experiments.
Butterfly effect and spatial structure of information spreading in a chaotic cellular automaton
S. W. Liu, J. Willsher, T. Bilitewski, J. J. Li, A. Smith, K. Christensen, R. Moessner, J. Knolle
Physical Review B 103 (9), 94109 (2021).
Inspired by recent developments in the study of chaos in many-body systems, we construct a measure of local information spreading for a stochastic cellular automaton in the form of a spatiotemporally resolved Hamming distance. This decorrelator is a classical version of an out-of-time-order correlator studied in the context of quantum many-body systems. Focusing on the one-dimensional Kauffman cellular automaton, we extract the scaling form of our decorrelator with an associated butterfly velocity vb and a velocity-dependent Lyapunov exponent lambda(v). The existence of the latter is not a given in a discrete classical system. Second, we account for the behavior of the decorrelator in a framework based solely on the boundary of the information spreading, including an effective boundary random walk model yielding the full functional form of the decorrelator. In particular, we obtain analytic results for v(b) and the exponent beta in the scaling ansatz lambda(v) similar to mu(v - v(b))(beta), which is usually only obtained numerically. Finally, a full scaling collapse establishes the decorrelator as a unifying diagnostic of information spreading.
Bistability and time crystals in long-ranged directed percolation
A. Pizzi, A. Nunnenkamp, J. Knolle
Nature Communications 12 (1), 1061 (2021).
Stochastic processes govern the time evolution of a huge variety of realistic systems throughout the sciences. A minimal description of noisy many-particle systems within a Markovian picture and with a notion of spatial dimension is given by probabilistic cellular automata, which typically feature time-independent and short-ranged update rules. Here, we propose a simple cellular automaton with power-law interactions that gives rise to a bistable phase of long-ranged directed percolation whose long-time behaviour is not only dictated by the system dynamics, but also by the initial conditions. In the presence of a periodic modulation of the update rules, we find that the system responds with a period larger than that of the modulation for an exponentially (in system size) long time. This breaking of discrete time translation symmetry of the underlying dynamics is enabled by a self-correcting mechanism of the long-ranged interactions which compensates noise-induced imperfections. Our work thus provides a firm example of a classical discrete time crystal phase of matter and paves the way for the study of novel non-equilibrium phases in the unexplored field of driven probabilistic cellular automata. A model of a classical discrete time crystal satisfying the criteria of persistent subharmonic response robust against thermal noise and defects has been lacking. Here, the authors show that these criteria are satisfied in one-dimensional probabilistic cellular automata with long-range interactions and bistability.
Seasonal epidemic spreading on small-world networks: Biennial outbreaks and classical discrete time crystals
D. Malz, A. Pizzi, A. Nunnenkamp, J. Knolle
Physical Review Research 3 (1), 13124 (2021).
We study seasonal epidemic spreading in a susceptible-infected-removed-susceptible model on small-world graphs. We derive a mean-field description that accurately captures the salient features of the model, most notably a phase transition between annual and biennial outbreaks. A numerical scaling analysis exhibits a diverging autocorrelation time in the thermodynamic limit, which confirms the presence of a classical discrete time crystalline phase. We derive the phase diagram of the model both frommean-field theory and from numerics. Our paper demonstrates that small worldness and non-Markovianity can stabilize a classical discrete time crystal, and links recent efforts to understand such dynamical phases of matter to the century-old problem of biennial epidemics.
Vacancy-Induced Low-Energy Density of States in the Kitaev Spin Liquid
W. H. Kao, J. Knolle, G. B. Halasz, R. Moessner, N. B. Perkins
Physical Review X 11 (1), 11034 (2021).
The Kitaev honeycomb model has attracted significant attention due to its exactly solvable spin-liquid ground state with fractionalized Majorana excitations and its possible materialization in magnetic Mott insulators with strong spin-orbit couplings. Recently, the 5d-electron compound H3LiIr2O6 has shown to be a strong candidate for Kitaev physics considering the absence of any signs of a long-range ordered magnetic state. In this work, we demonstrate that a finite density of random vacancies in the Kitaev model gives rise to a striking pileup of low-energy Majorana eigenmodes and reproduces the apparent power-law upturn in the specific heat measurements of H3LiIr2O6. Physically, the vacancies can originate from various sources such as missing magnetic moments or the presence of nonmagnetic impurities (true vacancies), or from local weak couplings of magnetic moments due to strong but rare bond randomness (quasivacancies). We show numerically that the vacancy effect is readily detectable even at low vacancy concentrations and that it is not very sensitive either to the nature of vacancies or to different flux backgrounds. We also study the response of the site-diluted Kitaev spin liquid to the three-spin interaction term, which breaks time-reversal symmetry and imitates an external magnetic field. We propose a field-induced flux-sector transition where the ground state becomes flux-free for larger fields, resulting in a clear suppression of the low-temperature specific heat. Finally, we discuss the effect of dangling Majorana fermions in the case of true vacancies and show that their coupling to an applied magnetic field via the Zeeman interaction can also account for the scaling behavior in the high-field limit observed in H3LiIr2O6.
Random Multipolar Driving: Tunably Slow Heating through Spectral Engineering
H. Z. Zhao, F. Mintert, R. Moessner, J. Knolle
Physical Review Letters 126 (4), 40601 (2021).
Driven quantum systems may realize novel phenomena absent in static systems, but driving-induced heating can limit the timescale on which these persist. We study heating in interacting quantum many-body systems driven by random sequences with n-multipolar correlations, corresponding to a polynomially suppressed low-frequency spectrum. For n >= 1, we find a prethermal regime, the lifetime of which grows algebraically with the driving rate, with exponent 2n + 1. A simple theory based on Fermi's golden rule accounts for this behavior. The quasiperiodic Thue-Morse sequence corresponds to the n -> infinity limit and, accordingly, exhibits an exponentially long-lived prethermal regime. Despite the absence of periodicity in the drive, and in spite of its eventual heat death, the prethermal regime can host versatile nonequilibrium phases, which we illustrate with a random multipolar discrete time crystal.
Time crystallinity and finite-size effects in clean Floquet systems
A. Pizzi, D. Malz, G. De Tomasi, J. Knolle, A. Nunnenkamp
Physical Review B 102 (21), 214207 (2020).
A cornerstone assumption that most literature on discrete time crystals has relied on is that homogeneous Floquet systems generally heat to a featureless infinite temperature state, an expectation that motivated researchers in the field to mostly focus on many-body localized systems. Some works have, however, shown that the standard diagnostics for time crystallinity apply equally well to clean settings without disorder. This fact raises the question whether a homogeneous discrete time crystal is possible in which the originally expected heating is evaded. Studying both a localized and an homogeneous model with short-range interactions, we clarify this issue showing explicitly the key differences between the two cases. On the one hand, our careful scaling analysis confirms that, in the thermodynamic limit and in contrast to localized discrete time crystals, homogeneous systems indeed heat. On the other hand, we show that, thanks to a mechanism reminiscent of quantum scars, finite-size homogeneous systems can still exhibit very crisp signatures of time crystallinity. A subharmonic response can in fact persist over timescales that are much larger than those set by the integrability-breaking terms, with thermalization possibly occurring only at very large system sizes (e.g., of hundreds of spins). Beyond clarifying the emergence of heating in disorder-free systems, our work casts a spotlight on finite-size homogeneous systems as prime candidates for the experimental implementation of nontrivial out-of-equilibrium physics.
Magneto-optical conductivity in generic Weyl semimetals
M. Stalhammar, J. Larana-Aragon, J. Knolle, E. J. Bergholtz
Physical Review B 102 (23), 235134 (2020).
Magneto-optical studies of Weyl semimetals have been proposed as a versatile tool for observing low-energy Weyl fermions in candidate materials including the chiral Landau level. However, previous theoretical results have been restricted to the linearized regime around the Weyl node and are at odds with experimental findings. Here, we derive a closed form expression for the magneto-optical conductivity of generic Weyl semimetals in the presence of an external magnetic field aligned with the tilt of the spectrum. The systems are taken to have linear dispersion in two directions, while the tilting direction can consist of any arbitrary continuously differentiable function. This general calculation is then used to analytically evaluate the magneto-optical conductivity of Weyl semimetals expanded to cubic order in momentum. In particular, systems with arbitrary tilt, as well as systems hosting trivial Fermi pockets are investigated. The higher-order terms in momentum close the Fermi pockets in the type-II regime, removing the need for unphysical cutoffs when evaluating the magneto-optical conductivity. Crucially, the ability to take into account closed over-tilted and additional trivial Fermi pockets allows us to treat model systems closer to actual materials and we propose a simple explanation why the presence of parasitic trivial Fermi pockets can mask the characteristic signature of Weyl fermions in magneto-optical conductivity measurements.
Disorder-free localization in a simple U (1) lattice gauge theory
I. Papaefstathiou, A. Smith, J. Knolle
Physical Review B 102 (16), 165132 (2020).
Localization due to the presence of disorder has proven crucial for our current understanding of relaxation in isolated quantum systems. The many-body localized phase constitutes a robust alternative to the thermalization of complex interacting systems, but recently the importance of disorder has been brought into question. A number of disorder-free localization mechanisms have been put forward connected to local symmetries of lattice gauge theories. Here, starting from translationally invariant (1 + 1)-dimensional quantum electrodynamics, we modify the dynamics of the gauge field which allows us to construct a lattice model with a U(1) local gauge symmetry revealing a mechanism of disorder-free localization. We consider two different discretizations of the continuum model resulting in a free-fermion soluble model in one case and an interacting model in the other. We diagnose the localization of our translationally invariant model in the far-from-equilibrium dynamics following a global quantum quench.
Local probes for charge-neutral edge states in two-dimensional quantum magnets
J. Feldmeier, W. Natori, M. Knap, J. Knolle
Physical Review B 102 (13), 134423 (2020).
The bulk-boundary correspondence is a defining feature of topological states of matter. However, for quantum magnets in two dimensions such as spin liquids or topological magnon insulators, a direct observation of topological surface states has proven challenging because of the charge-neutral character of the excitations. Here we propose spin-polarized scanning tunneling microscopy as a spin-sensitive local probe to provide direct information about charge-neutral topological edge states. We show how their signatures, imprinted in the local structure factor, can be extracted by specifically employing the strengths of existing technologies. As our main example, we determine the dynamical spin correlations of the Kitaev honeycomb model with open boundaries. We show that by contrasting conductance measurements of bulk and edge locations, one can extract direct signatures of the existence of fractionalized excitations and nontrivial topology. The broad applicability of this approach is corroborated by a second example of a kagome topological magnon insulator.
Dynamics of a Two-Dimensional Quantum Spin-Orbital Liquid: Spectroscopic Signatures of Fermionic Magnons
W. M. H. Natori, J. Knolle
Physical Review Letters 125 (6), 67201 (2020).
We provide an exact study of dynamical correlations for the quantum spin-orbital liquid phases of an SU(2)-symmetric Kitaev honeycomb lattice model. We show that the spin dynamics in this Kugel-Khomskii type model is exactly the density-density correlation function of S = 1 fermionic magnons, which could be probed in resonant inelastic x-ray scattering experiments. We predict the characteristic signatures of spin-orbital fractionalization in inelastic scattering experiments and compare them to the ones of the spin-anisotropic Kitaev honeycomb spin liquid. In particular, the resonant inelastic x-ray scattering response shows a characteristic momentum dependence directly related to the dispersion of fermionic excitations. The neutron scattering cross section displays a mixed response of fermionic magnons as well as spin-orbital excitations. The latter has a bandwidth of broad excitations and a vison gap that is three times larger than that of the spin-1 = 2 Kitaev model.
Quantum Many-Body Scars in Optical Lattices
H. Z. Zhao, J. Vovrosh, F. Mintert, J. Knolle
Physical Review Letters 124 (16), 160604 (2020).
The concept of quantum many-body scars has recently been put forward as a route to describe weak ergodicity breaking and violation of the eigenstate thermalization hypothesis. We propose a simple setup to generate quantum many-body scars in a doubly modulated Bose-Hubbard system which can be readily implemented in cold atomic gases. The dynamics are shown to be governed by kinetic constraints which appear via density-assisted tunneling in a high-frequency expansion. We find the optimal driving parameters for the kinetically constrained hopping which leads to small isolated subspaces of scared eigenstates. The experimental signatures and the transition to fully thermalizing behavior as a function of driving frequency are analyzed.
Electronic Properties of alpha-RuCl3 in Proximity to Graphene
S. Biswas, Y. Li, S. M. Winter, J. Knolle, R. Valenti
Physical Review Letters 123 (23), 237201 (2019).
In the pursuit of developing routes to enhance magnetic Kitaev interactions in alpha-RuCl3, as well as probing doping effects, we investigate the electronic properties of alpha-RuCl3 in proximity to graphene. We study alpha-RuCl3/graphene heterostructures via ab initio density functional theory calculations, Wannier projection, and nonperturbative exact diagonalization methods. We show that alpha-RuCl3 becomes strained when placed on graphene and charge transfer occurs between the two layers, making alpha-RuCl3 (graphene) lightly electron doped (hole doped). This gives rise to an insulator-to-metal transition in alpha-RuCl3 with the Fermi energy located close to the bottom of the upper Hubbard band of the t(2g) manifold. These results suggest the possibility of realizing metallic and even exotic superconducting states. Moreover, we show that in the strained alpha-RuCl3 monolayer the Kitaev interactions are enhanced by more than 50% compared to the unstrained bulk structure. Finally, we discuss scenarios related to transport experiments in alpha-RuCl3/graphene heterostructures.
Period-n Discrete Time Crystals and Quasicrystals with Ultracold Bosons
A. Pizzi, J. Knolle, A. Nunnenkamp
Physical Review Letters 123 (15), 150601 (2019).
"We investigate the out-of-equilibrium properties of a system of interacting bosons in a ring lattice. We present a Floquet driving that induces clockwise (counterclockwise) circulation of the particles among the odd (even) sites of the ring which can be mapped to a fully connected model of clocks of two counterrotating species. The clocklike motion of the particles is at the core of a period-n discrete time crystal where L = 2n is the number of lattice sites. In the presence of a ""staircaselike"" on-site potential, we report the emergence of a second characteristic timescale in addition to the period n-tupling. This new timescale depends on the microscopic parameters of the Hamiltonian and is incommensurate with the Floquet period, underpinning a dynamical phase we call ""time quasicrystal."" The rich dynamical phase diagram also features a thermal phase and an oscillatory phase, all of which we investigate and characterize. Our simple, yet rich model can be realized with state-of-the-art ultracold atoms experiments."